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Ambiguous - Kill la Kill OP2
God I love this opening so goddamn much. Seeing it for the first time was a really refreshing breath from the subpar first opening, especially since the quality and tone of the show was kinda way above the original's by this point. And Garnidelia. I mean. Garnidelia.
Futuristic Imagination - Eden of the East
Like the show, not really a fan of the English or Japanese openings, but I absolutely love Futuristic Imagination. This is the ending that immediately shoots to mind when it comes to making a list of favorites, so it's the one I'll post. The singer's fantastic and the song and creative visuals meld together really well and go along with the overall flow of the show.